Monte Carlo investigation of a kinetic Ising Model of the glass transition.

01 January 1986

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A detailed Monte Carlo study of the equilibrium and dynamical properties of the two-spin facilitated kinetic Ising model proposed by Fredrickson and Anderson (FA) is presented. The model Hamiltonian is that of a spin-1/2 Ising model in an external magnetic field and, in the present study, contains no interactions between spins. The kinetic properties of the model are described by a master equation with single-spin-flip dynamics and high cooperative flip rates. In particular, the rate at which spin flips is chosen to be zero unless at least two of its neighbors are spin up. Monte Carlo simulations of the model on a square lattice demonstrate that although there is no evidence for a kinetic singularity (as predicted by FA), the model has dynamical properties much like those of viscous liquids. We find non- Arrhenius temperature dependence of the average relaxation time and highly nonexponential decay of various relaxation functions.