Inhomogeneous CuO6 tilt distribution and charge-spin correlations in La2-x-yNdySrxCuO4 around the commensurate hole concentration

01 August 2003

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Phononic and magnetic Raman scattering are studied in La2-x-yNdySrxCuO4 with three doping concentrations: xapproximate to1/8, y=0; xapproximate to1/8, y=0.4; and x=0.01, y=0. We observe strong disorder in the tilt pattern of the CuO6 octahedra in both the orthorhombic and tetragonal phases that persist down to 10 K and are coupled to bond disorder in the cation layers around 1/8 doping independent of Nd concentration. The weak magnitude of existing charge-spin modulations in the Nd-doped structure does not allow us to detect the specific Raman signatures of lattice dynamics or two-magnon scattering around 2200 cm(-1).